Triggered self-assembly of magnetic nanoparticles
Identifieur interne : 000006 ( Main/Exploration ); précédent : 000005; suivant : 000007Triggered self-assembly of magnetic nanoparticles
Auteurs : L. Ye [États-Unis] ; T. Pearson [États-Unis] ; Y. Cordeau [États-Unis] ; O. T. Mefford [États-Unis] ; T. M. Crawford [États-Unis]Source :
- Scientific Reports [ 2045-2322 ] ; 2016.
Abstract
Colloidal magnetic nanoparticles are candidates for application in biology, medicine and nanomanufac-turing. Understanding how these particles interact collectively in fluids, especially how they assemble and aggregate under external magnetic fields, is critical for high quality, safe, and reliable deployment of these particles. Here, by applying magnetic forces that vary strongly over the same length scale as the colloidal stabilizing force and then varying this colloidal repulsion, we can trigger self-assembly of these nanoparticles into parallel line patterns on the surface of a disk drive medium. Localized within nanometers of the medium surface, this effect is strongly dependent on the ionic properties of the colloidal fluid but at a level too small to cause bulk colloidal aggregation. We use real-time optical diffraction to monitor the dynamics of self-assembly, detecting local colloidal changes with greatly enhanced sensitivity compared with conventional light scattering. Simulations predict the triggering but not the dynamics, especially at short measurement times. Beyond using spatially-varying magnetic forces to balance interactions and drive assembly in magnetic nanoparticles, future measurements leveraging the sensitivity of this approach could identify novel colloidal effects that impact real-world applications of these nanoparticles.
Url:
DOI: 10.1038/srep23145
PubMed: 26975332
PubMed Central: 4791594
Affiliations:
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Ye</name><affiliation wicri:level="1"><nlm:aff id="a1"><institution>Smart State Center for Experimental Nanoscale Physics and Department of Physics and Astronomy, University of South Carolina</institution>, Columbia, SC 29208,<country>USA</country></nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation><affiliation wicri:level="1"><nlm:aff id="a3"><institution>Present Address: MagAssemble LLC</institution>, Irmo, SC 29063<country>USA</country></nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Pearson, T" sort="Pearson, T" uniqKey="Pearson T" first="T." last="Pearson">T. Pearson</name><affiliation wicri:level="1"><nlm:aff id="a1"><institution>Smart State Center for Experimental Nanoscale Physics and Department of Physics and Astronomy, University of South Carolina</institution>, Columbia, SC 29208,<country>USA</country></nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Cordeau, Y" sort="Cordeau, Y" uniqKey="Cordeau Y" first="Y." last="Cordeau">Y. Cordeau</name><affiliation wicri:level="1"><nlm:aff id="a2"><institution>Center for Optical Materials Science and Engineering Technologies (COMSET) and Department of Materials Science and Engineering, Clemson University</institution>, 161 Sirrine Hall, Clemson, SC 29634<country>USA</country></nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Mefford, O T" sort="Mefford, O T" uniqKey="Mefford O" first="O. T." last="Mefford">O. T. Mefford</name><affiliation wicri:level="1"><nlm:aff id="a2"><institution>Center for Optical Materials Science and Engineering Technologies (COMSET) and Department of Materials Science and Engineering, Clemson University</institution>, 161 Sirrine Hall, Clemson, SC 29634<country>USA</country></nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Crawford, T M" sort="Crawford, T M" uniqKey="Crawford T" first="T. M." last="Crawford">T. M. Crawford</name><affiliation wicri:level="1"><nlm:aff id="a1"><institution>Smart State Center for Experimental Nanoscale Physics and Department of Physics and Astronomy, University of South Carolina</institution>, Columbia, SC 29208,<country>USA</country></nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author></analytic><series><title level="j">Scientific Reports</title><idno type="eISSN">2045-2322</idno><imprint><date when="2016">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>Colloidal magnetic nanoparticles are candidates for application in biology, medicine and nanomanufac-turing. Understanding how these particles interact collectively in fluids, especially how they assemble and aggregate under external magnetic fields, is critical for high quality, safe, and reliable deployment of these particles. Here, by applying magnetic forces that vary strongly over the same length scale as the colloidal stabilizing force and then varying this colloidal repulsion, we can trigger self-assembly of these nanoparticles into parallel line patterns on the surface of a disk drive medium. Localized within nanometers of the medium surface, this effect is strongly dependent on the ionic properties of the colloidal fluid but at a level too small to cause bulk colloidal aggregation. We use real-time optical diffraction to monitor the dynamics of self-assembly, detecting local colloidal changes with greatly enhanced sensitivity compared with conventional light scattering. Simulations predict the triggering but not the dynamics, especially at short measurement times. Beyond using spatially-varying magnetic forces to balance interactions and drive assembly in magnetic nanoparticles, future measurements leveraging the sensitivity of this approach could identify novel colloidal effects that impact real-world applications of these nanoparticles.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Pankhurst, Q A" uniqKey="Pankhurst Q">Q. A. Pankhurst</name></author><author><name sortKey="Connolly, J" uniqKey="Connolly J">J. Connolly</name></author><author><name sortKey="Jones, S" uniqKey="Jones S">S. Jones</name></author><author><name sortKey="Dobson, J" uniqKey="Dobson J">J. Dobson</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Pankhurst, Q A" uniqKey="Pankhurst Q">Q. A. Pankhurst</name></author><author><name sortKey="Thanh, N T K" uniqKey="Thanh N">N. T. K. Thanh</name></author><author><name sortKey="Jones, S K" uniqKey="Jones S">S. K. 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Weaver</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Xue, X" uniqKey="Xue X">X. Xue</name></author><author><name sortKey="Wang, J" uniqKey="Wang J">J. Wang</name></author><author><name sortKey="Furlani, E P" uniqKey="Furlani E">E. P. Furlani</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Furlani, E" uniqKey="Furlani E">E. Furlani</name></author><author><name sortKey="Ng, K" uniqKey="Ng K">K. Ng</name></author></analytic></biblStruct></listBibl></div1></back></TEI><affiliations><list><country><li>États-Unis</li></country></list><tree><country name="États-Unis"><noRegion><name sortKey="Ye, L" sort="Ye, L" uniqKey="Ye L" first="L." last="Ye">L. Ye</name></noRegion><name sortKey="Cordeau, Y" sort="Cordeau, Y" uniqKey="Cordeau Y" first="Y." last="Cordeau">Y. Cordeau</name><name sortKey="Crawford, T M" sort="Crawford, T M" uniqKey="Crawford T" first="T. M." last="Crawford">T. M. Crawford</name><name sortKey="Mefford, O T" sort="Mefford, O T" uniqKey="Mefford O" first="O. T." last="Mefford">O. T. Mefford</name><name sortKey="Pearson, T" sort="Pearson, T" uniqKey="Pearson T" first="T." last="Pearson">T. Pearson</name><name sortKey="Ye, L" sort="Ye, L" uniqKey="Ye L" first="L." last="Ye">L. Ye</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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